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The results are as follows:1 No significant difference in the translational energy distributions for different CO rotational state products has been observed at 208nm and 213nm excitation wavelengths.

主要结论如下:(1)光解碎片CO 在208nm、213nm 两个解离波长下不同振转态的平动能分布没有明显地差别,而其不同振转态的各向异性参数β却有明显地不同。

Product translational energy distribution and angular anisotropydistribution for the CH_2 product from CH3 photodissociation at differentvibrational levels via the 3s Rydberg state have been measured.

我们测量了不同的振动态的CH3 自由基3s 里德堡态的解离产物H 原子的时间飞行谱,从而得到解离产物的平动能分布。

In the collisional energy transfer process Cs(6P3/2)+(Ne,N2), it is possible that the electronic state merely transfer to the translational energy for Ne.

在CS(6P3/2)+(Ne, N2)碰撞能量转移过程对于6P3/2与Ne的碰撞,电子态能量仅能转移为Ne原子的平动能

We mainly detected the TOF and angular distribution of photofragment, and get the anisotropy parameter β and the translational energy distribution. In addition, we calculated the geometries of the ground states, the excited states and the triplet excited states, and the transition electric dipole moments. According to these, the dissociation lifetimes of some molecules are calculated.

主要是探测了光解碎片的时间飞渡谱和角分布并通过前向卷积方法拟合得到了各向异性参数β和光解碎片的平动能分布;此外还用从头计算方法计算了反应物分子的基态、激发态、三重激发态的平衡几何构型和分子的跃迁偶极矩并据此计算了一部分分子的解离态寿命。

The N + OH reaction system has no energy barrier in the entrance channel on the PES; instead, there are double wells along the reaction path, which leads to that the integral reaction cross sections are not strongly dependent on either translational energy or initial rotational and vibrational state.

计算还显示,由于N+OH反应入口谷没有能垒,而沿着最小能量反应路径有两个势阱,因此反应的积分截面并不强烈依赖平动能和反应物分子的初始振转态。

The mechanism studies on the atomic oxygen effects over surface materials become rather difficult due to the fact that the interaction, stemming from a highly complex environment in LEO, where the atomic oxygen are equipping with high translational kinetic energy and strong oxidizing characteristics, may induce complicated physico-chemical processes.

然而,由于空间环境高度复杂,以及环境中原子氧具有高平动能和高度活泼的化学特性,空间材料的原子氧效应呈现复杂的物理化学过程,给该效应的机理性研究带来严重困难。

M. translational distribution, angular distribution, and the branching ratios for different possible product channels by measuring the angle-resolved time of flight spectra of photofragments. Information about photodissociation processes such as dissociative lifetime of parent molecule, the orientation of transition dipole moment, and the symmetry change of the highly excited states can be deduced from the translational energy distribution and angular distribution.

碎片平动能谱方法是在无碰撞条件下研究光解动力学的一种理想方法,它通过测量光致碎片在不同角度的时间飞渡谱(Time of Flight,简称TOF),可以得到光解碎片质心系的平动能分布、角分布和不同解离通道之间的分支比等,由此可以推知母分子的解离寿命、跃迁偶极距的取向以及激发态分子的对称性变化等过渡态的动力学信息。

A two dimensional photofragment ion-velocity imaging technique coupled with a (2+1) resonance-enhanced multiphoton ionization scheme was utilized to obtain the angular and translational energy distributions of the nascent Br(2 P 3/2) and Br*(2 P 1/2) atoms.

实验中得到了二溴甲烷光解产生的Br*(2 P 1/2)和Br(2 P 3/2)在不同波长下的角度和平动能分布。

Photofragment translational spectroscopy is an ideal tool to investigate photodissociation dynamics under collision-free conditions through which one can obtain the total center of mass translational distribution, angular distribution, and the branching ratios for different possible product channels by measuring the angle-resolved time of flight spectra of photofragments. Information about photodissociation processes such as dissociative lifetime of parent molecule, the orientation of transition dipole moment, and the symmetry change of the highly excited states can be deduced from the translational energy distribution and angular distribution.

碎片平动能谱方法是在无碰撞条件下研究光解动力学的一种理想方法,它通过测量光致碎片在不同角度的时间飞渡谱(Time of Flight,简称TOF),可以得到光解碎片质心系的平动能分布、角分布和不同解离通道之间的分支比等,由此可以推知母分子的解离寿命、跃迁偶极距的取向以及激发态分子的对称性变化等过渡态的动力学信息。

A two dimensional photofragment ion-velocity imaging technique coupled with a (2+1) resonance-enhanced multiphoton ionization scheme was utilized to obtain the angular and translational energy distributions of the nascent Br2P(subscript 3/2 and Br(superscript *)2P(subscript 1/2 atoms.

实验中得到了二溴甲烷光解产生的Br2P(下标 1-2和Br2P(下标 3-2在不同波长下的角度和平动能分布。

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